Polybrominated diphenyl ethers in precipitation in Southern Sweden (Skåne, Lund)
作者： Arnout F.H ter Schure , Per Larsson
DOI: 10.1016/S1352-2310(02)00360-6
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摘要: The presence of polybrominated diphenyl ether (PBDE) flame retardants in total deposition (wet + dry) was assessed with the simultaneous use three bulk samplers during a 2 week period. particle associated and 'dissolved' phase were separated sampling. Volume weighted mean (VWM) concentrations SigmaPBDE (9 congeners) rain 209 pg l(-1). Total rates +/- 1 ng m(-2) day(-1). PBDE dominated by decaBDE(209) thereafter 2,2'4,4'-tetraBDE(47) 2,2'4,4',5-pentaBDE(99). Concentrations PBDEs used to calculate filter/adsorbent ratios (F/A). We found that 65 18% associated. Low F/A for higher brominated congeners (Br > 5) observed. This is contradictory predictions based on PBDEs' physico-chemical properties attributed sampling artefacts, such as size distribution, and/or non-equilibrium processes. There negative relationship between particulate concentration volume suggesting dilution effect importance scavenging wet PBDEs. (C) 2002 Elsevier Science Ltd. All rights reserved. (Less)
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P. Harding-Jones, Crispin J. Halsall, Kevin C. Jones, P. J. Coleman, V. Burnett, R. G. M. Lee, PCBs in UK urban air. ,(1995)
Jacob de Boer, Peter G. Wester, Hans J. C. Klamer, Wilma E. Lewis, Jan P. Boon, Do flame retardants threaten ocean life Nature. ,vol. 394, pp. 28- 29 ,(1998) , 10.1038/27798
L. Van Vaeck, G. Broddin, K. Van Cauwenberghe, Differences in particle size distributions of major organic pollutants in ambient aerosols in urban, rural, and seashore areas Environmental Science & Technology. ,vol. 13, pp. 1494- 1502 ,(1979) , 10.1021/ES60160A013
P Pistikopoulos, H.M Wortham, L Gomes, S Masclet-Beyne, E Bon Nguyen, P.A Masclet, G Mouvier, Mechanisms of formation of particulate polycyclic aromatic hydrocarbons in relation to the particle size distribution; effects on meso-scale transport Atmospheric Environment. Part A. General Topics. ,vol. 24, pp. 2573- 2584 ,(1990) , 10.1016/0960-1686(90)90135-A
Gian Marco Currado, Stuart Harrad, Factors Influencing Atmospheric Concentrations of Polychlorinated Biphenyls in Birmingham, U.K. Environmental Science & Technology. ,vol. 34, pp. 78- 82 ,(2000) , 10.1021/ES990752X
Peter S. Haglund, Douglas R. Zook, Hans-Rudolf Buser, Jiwei Hu, Identification and Quantification of Polybrominated Diphenyl Ethers and Methoxy-Polybrominated Diphenyl Ethers in Baltic Biota Environmental Science & Technology. ,vol. 31, pp. 3281- 3287 ,(1997) , 10.1021/ES9702834
D. E. Glotfelty, J. N. Seiber, A. Liljedahl, Pesticides in fog. Nature. ,vol. 325, pp. 602- 605 ,(1987) , 10.1038/325602A0
Carolyn J. Koester, Ronald A. Hites, Wet and dry deposition of chlorinated dioxins and furans Environmental Science & Technology. ,vol. 26, pp. 1375- 1382 ,(1992) , 10.1021/ES00031A015
Steven J. Eisenreich, Brian B. Looney, J. David. Thornton, Airborne organic contaminants in the Great Lakes ecosystem Environmental Science & Technology. ,vol. 15, pp. 30- 38 ,(1981) , 10.1021/ES00083A002
Gulbrand Lunde, Jørgen Gether, Nina Gjøs, May-Berit Støbet Lande, Organic micropollutants in precipitation in Norway Atmospheric Environment. ,vol. 11, pp. 1007- 1014 ,(1977) , 10.1016/0004-6981(77)90229-3