Pliable polaritons: Wannier exciton-plasmon coupling in metal-semiconductor structures

作者: Jacob B. Khurgin

DOI: 10.1515/NANOPH-2018-0166

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摘要: Plasmonic structures are known to support the modes with subwavelength volumes in which field matter interactions greatly enhanced. Coupling between molecular excitations and plasmons leading formation of plexcitons has been investigated for a number organic molecules. However, plasmon-exciton coupling metal semiconductor have not experienced same degree attention. In this work we show that very strong regime Rabi energy exceeds exciton binding is attainable cladded plasmonic nanoparticles leads Wannier Exciton Plasmon Polariton (WEPP) bound nanoparticle characterized by dramatically smaller (by factor few) excitonic radius correspondingly higher ionization energy. This exceeding approaching 100meV CdS/Ag may make room temperature Bose Einstein condensation polariton lasing plasmonic/semiconductor possible

参考文章(48)
H. Fröhlich, Electrons in lattice fields Advances in Physics. ,vol. 3, pp. 325- 361 ,(1954) , 10.1080/00018735400101213
A. Huber, N. Ocelic, D. Kazantsev, R. Hillenbrand, Near-field imaging of mid-infrared surface phonon polariton propagation Applied Physics Letters. ,vol. 87, pp. 081103- ,(2005) , 10.1063/1.2032595
Hao Zhang, Na Young Kim, Yoshihisa Yamamoto, Neil Na, Very strong coupling in GaAs-based optical microcavities Physical Review B. ,vol. 87, pp. 115303- ,(2013) , 10.1103/PHYSREVB.87.115303
J. Frenkel, On the Transformation of light into Heat in Solids. I Physical Review. ,vol. 37, pp. 17- 44 ,(1931) , 10.1103/PHYSREV.37.17
Nche T. Fofang, Tae-Ho Park, Oara Neumann, Nikolay A. Mirin, Peter Nordlander, Naomi J. Halas, Plexcitonic nanoparticles: plasmon-exciton coupling in nanoshell-J-aggregate complexes. Nano Letters. ,vol. 8, pp. 3481- 3487 ,(2008) , 10.1021/NL8024278
D. S. Citrin, J. B. Khurgin, Microcavity effect on the electron-hole relative motion in semiconductor quantum wells Physical Review B. ,vol. 68, pp. 205325- ,(2003) , 10.1103/PHYSREVB.68.205325
Michael Claybourn, Michael D. Scott, John O. Williams, Robert C. Goodfellow, Epitaxial growth of CdS and CdS1−ySey thin films by hydrogen transport from the elements and their photoluminescent properties Journal of Crystal Growth. ,vol. 58, pp. 417- 424 ,(1982) , 10.1016/0022-0248(82)90290-1
Y. Todorov, A. M. Andrews, R. Colombelli, S. De Liberato, C. Ciuti, P. Klang, G. Strasser, C. Sirtori, Ultrastrong light-matter coupling regime with polariton dots. Physical Review Letters. ,vol. 105, pp. 196402- 196402 ,(2010) , 10.1103/PHYSREVLETT.105.196402
Jacob B. Khurgin, Greg Sun, Scaling of losses with size and wavelength in nanoplasmonics and metamaterials Applied Physics Letters. ,vol. 99, pp. 211106- ,(2011) , 10.1063/1.3664105