Direct optical excitation of a fullerene-incarcerated metal ion
作者： Mark A.G. Jones , R.A. Taylor , A. Ardavan , K. Porfyrakis , G.A.D. Briggs
DOI: 10.1016/J.CPLETT.2006.06.094
关键词:
摘要: Abstract The endohedral fullerene Er 3 N@C 80 shows characteristic 1.5 μm photoluminescence at cryogenic temperatures associated with radiative relaxation from the crystal-field split 3+ 4 I 13/2 manifold to 15/2 manifold. Previous observations of this luminescence were carried out by photoexcitation cage states leading via ionic states. We present direct non-cage-mediated optical interaction erbium ion. have used complete a photoluminescence-excitation map This ability interact directly an incarcerated ion suggests possibility coherently manipulating qubit light.
harvard.edu
arxiv.org
elsevier.com
sci-hub.se 参考文章(8)
S. Stevenson, G. Rice, T. Glass, K. Harich, F. Cromer, M. R. Jordan, J. Craft, E. Hadju, R. Bible, M. M. Olmstead, K. Maitra, A. J. Fisher, A. L. Balch, H. C. Dorn, Small-bandgap endohedral metallofullerenes in high yield and purity Nature. ,vol. 401, pp. 55- 57 ,(1999) , 10.1038/43415
Wolfgang Harneit, Fullerene-based electron-spin quantum computer Physical Review A. ,vol. 65, pp. 032322- ,(2002) , 10.1103/PHYSREVA.65.032322
Henry. Ajie, Marcos M. Alvarez, Samir J. Anz, Rainer D. Beck, Francois. Diederich, K. Fostiropoulos, Donald R. Huffman, Wolfgang. Kraetschmer, Yves. Rubin, . et al., Characterization of the soluble all-carbon molecules C60 and C70 The Journal of Physical Chemistry. ,vol. 94, pp. 8630- 8633 ,(1990) , 10.1021/J100387A004
Michael F. Reid, F. S. Richardson, Electric dipole intensity parameters for lanthanide 4f → 4f transitions The Journal of Chemical Physics. ,vol. 79, pp. 5735- 5742 ,(1983) , 10.1063/1.445760
R.M. Macfarlane, D. S Bethune, S. Stevenson, H.C. Dorn, Fluorescence spectroscopy and emission lifetimes of Er3+ in Er Sc3−N@C80 (x=1–3) Chemical Physics Letters. ,vol. 343, pp. 229- 234 ,(2001) , 10.1016/S0009-2614(01)00701-1
Simon C Benjamin, Arzhang Ardavan, G Andrew D Briggs, David A Britz, Daniel Gunlycke, John Jefferson, Mark A G Jones, David F Leigh, Brendon W Lovett, Andrei N Khlobystov, S A Lyon, John J L Morton, Kyriakos Porfyrakis, Mark R Sambrook, Alexei M Tyryshkin, Towards a fullerene-based quantum computer Journal of Physics: Condensed Matter. ,vol. 18, ,(2006) , 10.1088/0953-8984/18/21/S12
A. Ardavan, M. Austwick, S. C. Benjamin, G. A. D. Briggs, T. J. S. Denni s, A. Ferguson, D. G. Hasko, M. Kanai, A. N. Khlobystov, B. W. Lovett, G. W. Morley, R. A. Oliver, D. G. Pettifor, K. Porfyrakis, J. H. Reina, J. H. Rice, J. D. Smith, R. A. Taylor, D. A. Williams, C. Adelmann, H. Mariette, R. J. Hamers, Nanoscale solid-state quantum computing Philosophical Transactions of the Royal Society A. ,vol. 361, pp. 1473- 1485 ,(2003) , 10.1098/RSTA.2003.1214
Roger M. Macfarlane, Georg Wittmann, Paul H. M. van Loosdrecht, Mattanjah de Vries, Donald S. Bethune, Steve Stevenson, Harry C. Dorn, Measurement of Pair Interactions and1.5μmEmission fromEr3+Ions in aC82Fullerene Cage Physical Review Letters. ,vol. 79, pp. 1397- 1400 ,(1997) , 10.1103/PHYSREVLETT.79.1397