Investigation of the rotational dynamics in liquids by time-resolved cars

作者: N. Kohles , A. Laubereau

DOI: 10.1016/0009-2614(87)80400-1

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摘要: Abstract The asymptotic decay time τ an of the anisotropic vibrational excitation in liquids has been measured for first time-resolved CARS. use different polarization geometries also allows us to determine orientational relaxation R . Experimental data are presented totally symmetric modes liquid CS 2 and CH 3 I, where describes “tumbling” motion symmetry axis.

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