Visualizing Exotic Orbital Texture in the Single-Layer Mott Insulator 1T-TaSe2

作者: Oliver R. Albertini , Jonathan A. Sobota , Zhi-Xun Shen , Yi Chen , Hyejin Ryu

DOI: 10.1038/S41567-019-0744-9

关键词:

摘要: Mott insulating behavior is induced by strong electron correlation and can lead to exotic states of matter such as unconventional superconductivity quantum spin liquids. Recent advances in van der Waals material synthesis enable the exploration novel systems two-dimensional limit. Here we report characterization local electronic properties single- few-layer 1T-TaSe2 via spatial- momentum-resolved spectroscopy involving scanning tunneling microscopy angle-resolved photoemission. Our combined experimental theoretical study indicates that induces a robust insulator state single-layer accompanied orbital texture. Inclusion interlayer coupling weakens phase 1T-TaSe2, seen reduction its energy gap quenching correlation-driven texture bilayer trilayer 1T-TaSe2. results establish useful new platform for investigating physics two dimensions.

参考文章(54)
Chris A. Marianetti, Pierre Darancet, Andrew J. Millis, Three-dimensional metallic and two-dimensional insulating behavior in octahedral tantalum dichalcogenides Physical Review B. ,vol. 90, pp. 045134- ,(2014) , 10.1103/PHYSREVB.90.045134
Martin Schlipf, François Gygi, Optimization Algorithm for the Generation of ONCV Pseudopotentials Computer Physics Communications. ,vol. 196, pp. 36- 44 ,(2015) , 10.1016/J.CPC.2015.05.011
Stefano Colonna, Fabio Ronci, Antonio Cricenti, Luca Perfetti, Helmuth Berger, Marco Grioni, Mott phase at the surface of 1T-TaSe2 observed by scanning tunneling microscopy. Physical Review Letters. ,vol. 94, pp. 036405- ,(2005) , 10.1103/PHYSREVLETT.94.036405
Qingyan Wang, Wenhao Zhang, Lili Wang, Ke He, Xucun Ma, Qikun Xue, Large-scale uniform bilayer graphene prepared by vacuum graphitization of 6H-SiC(0001) substrates. Journal of Physics: Condensed Matter. ,vol. 25, pp. 095002- 095002 ,(2013) , 10.1088/0953-8984/25/9/095002
C. Sohrt, A. Stange, M. Bauer, K. Rossnagel, How fast can a Peierls-Mott insulator be melted? Faraday Discussions. ,vol. 171, pp. 243- 257 ,(2014) , 10.1039/C4FD00042K
F.J. Di Salvo, R.G. Maines, J.V. Waszczak, R.E. Schwall, Preparation and properties of 1TTaSe2 Solid State Communications. ,vol. 14, pp. 497- 501 ,(1974) , 10.1016/0038-1098(74)90975-2
T. Ritschel, J. Trinckauf, K. Koepernik, B. Büchner, M. v. Zimmermann, H. Berger, Y. I. Joe, P. Abbamonte, J. Geck, Orbital textures and charge density waves in transition metal dichalcogenides Nature Physics. ,vol. 11, pp. 328- 331 ,(2015) , 10.1038/NPHYS3267
John P. Perdew, Kieron Burke, Matthias Ernzerhof, Generalized Gradient Approximation Made Simple Physical Review Letters. ,vol. 77, pp. 3865- 3868 ,(1996) , 10.1103/PHYSREVLETT.77.3865
R. Brouwer, F. Jellinek, LOW-TEMPERATURE SUPERSTRUCTURES OF 1T-TASE2 AND 2H-TASE2 Physica B-condensed Matter. ,vol. 99, pp. 51- 55 ,(1980) , 10.1016/0378-4363(80)90209-0
S. L. Dudarev, G. A. Botton, S. Y. Savrasov, C. J. Humphreys, A. P. Sutton, Electron-energy-loss spectra and the structural stability of nickel oxide: An LSDA+U study Physical Review B. ,vol. 57, pp. 1505- 1509 ,(1998) , 10.1103/PHYSREVB.57.1505