Transient coherent Raman scattering in the time and frequency domain

作者: W. Zinth

DOI: 10.1016/0030-4018(80)90421-6

关键词:

摘要: A new type of Raman spectroscopy is presented: After transient excitation molecular modes coherently scattered spectra are investigated in a depayed probing experiment. The spectral position the mode observed after long delay times. dephasing time obtained from dependence amplitudes. Frequency disturbing non-resonant susceptibilities eliminated. We report on first experimental results coherent liquid CH3CCl3.

参考文章(12)
J. J. Song, G. L. Eesley, M. D. Levenson, Background suppression in coherent Raman spectroscopy Applied Physics Letters. ,vol. 29, pp. 567- 569 ,(1976) , 10.1063/1.89189
A. Laubereau, W. Kaiser, Vibrational dynamics of liquids and solids investigated by picosecond light pulses Reviews of Modern Physics. ,vol. 50, pp. 607- 665 ,(1978) , 10.1103/REVMODPHYS.50.607
W. Zinth, A. Laibereau, W. Kaiser, Generation of chirp-free picosecond pulses Optics Communications. ,vol. 22, pp. 161- 164 ,(1977) , 10.1016/0030-4018(77)90010-4
R. L. Carman, F. Shimizu, C. S. Wang, N. Bloembergen, Theory of Stokes Pulse Shapes in Transient Stimulated Raman Scattering Physical Review A. ,vol. 2, pp. 60- 72 ,(1970) , 10.1103/PHYSREVA.2.60
W. Zinth, A. Laubereau, W. Kaiser, Time resolved observation of resonant and non-resonant contributions to the nonlinear susceptibility χ(3) Optics Communications. ,vol. 26, pp. 457- 462 ,(1978) , 10.1016/0030-4018(78)90246-8
S.A. Akhmanov, Transient effects in stimulated Raman scattering Materials Research Bulletin. ,vol. 4, pp. 455- 462 ,(1969) , 10.1016/0025-5408(69)90104-4
A. Laubereau, G. Wochner, W. Kaiser, Ultrafast coherent excitation and probing of molecular vibrations with isotopic substructure Physical Review A. ,vol. 13, pp. 2212- 2225 ,(1976) , 10.1103/PHYSREVA.13.2212
A. Penzkofer, A. Laubereau, W. Kaiser, High intensity Raman interactions Progress in Quantum Electronics. ,vol. 6, pp. 55- 140 ,(1979) , 10.1016/0079-6727(79)90011-9