A comparative investigation of H 2 O 2 -involved pretreatments on lignocellulosic biomass for enzymatic hydrolysis

作者: Maoyuan Luo , Dong Tian , Fei Shen , Jinguang Hu , Yanzong Zhang

DOI: 10.1007/S13399-018-0364-0

关键词:

摘要: An effective pretreatment to improve cellulose accessibility and facilitate glucose release is crucial in a cellulosic ethanol biorefinery. This work comparatively assessed four H2O2-involved pretreatments, i.e., concentrated H3PO4 plus H2O2 (PHP), H2O2–CH3COOH (HPAC), alkaline-H2O2 (AHP), Fenton chemistry (FC), for their performances on wheat straw, poplar, birch biomass. Substrate characteristics before after were using SEM, XRD, LSCM. The hydrolytic potentials of the pretreated substrates compared by Simons’ stain cellulose–glucose conversion assessment. results showed that acidic pretreatments (PHP HPAC) more efficient biomass delignification AHP FC. PHP promising production due its corresponding high yield (368.0 mg g−1) enzymatic hydrolysis.

参考文章(47)
Jingwen Qiu, Qing Wang, Fei Shen, Gang Yang, Yanzong Zhang, Shihuai Deng, Jing Zhang, Yongmei Zeng, Chun Song, Optimizing Phosphoric Acid plus Hydrogen Peroxide (PHP) Pretreatment on Wheat Straw by Response Surface Method for Enzymatic Saccharification Applied Biochemistry and Biotechnology. ,vol. 181, pp. 1123- 1139 ,(2017) , 10.1007/S12010-016-2273-7
Benjamin Martin, Joerg Sedelmeier, Anaïs Bouisseau, Patricia Fernandez-Rodriguez, Julien Haber, Florian Kleinbeck, Sonja Kamptmann, Flavien Susanne, Pascale Hoehn, Marian Lanz, Laurent Pellegatti, Francesco Venturoni, Jeremy Robertson, Michael C. Willis, Berthold Schenkel, Toolbox study for application of hydrogen peroxide as a versatile, safe and industrially-relevant green oxidant in continuous flow mode Green Chemistry. ,vol. 19, pp. 1439- 1448 ,(2017) , 10.1039/C6GC02899C
Dong Tian, Jinguang Hu, Richard P. Chandra, Jack N. Saddler, Canhui Lu, Valorizing Recalcitrant Cellulolytic Enzyme Lignin via Lignin Nanoparticles Fabrication in an Integrated Biorefinery ACS Sustainable Chemistry & Engineering. ,vol. 5, pp. 2702- 2710 ,(2017) , 10.1021/ACSSUSCHEMENG.6B03043
Jingwen Qiu, Lunjie Ma, Fei Shen, Gang Yang, Yanzong Zhang, Shihuai Deng, Jing Zhang, Yongmei Zeng, Yaodong Hu, Pretreating wheat straw by phosphoric acid plus hydrogen peroxide for enzymatic saccharification and ethanol production at high solid loading Bioresource Technology. ,vol. 238, pp. 174- 181 ,(2017) , 10.1016/J.BIORTECH.2017.04.040
Christos Didaskalou, Sibel Buyuktiryaki, Rustem Kecili, Claudio P. Fonte, Gyorgy Szekely, Valorisation of agricultural waste with an adsorption/nanofiltration hybrid process: from materials to sustainable process design Green Chemistry. ,vol. 19, pp. 3116- 3125 ,(2017) , 10.1039/C7GC00912G
Dong Tian, Richard P. Chandra, Jin-Suk Lee, Canhui Lu, Jack N. Saddler, A comparison of various lignin-extraction methods to enhance the accessibility and ease of enzymatic hydrolysis of the cellulosic component of steam-pretreated poplar. Biotechnology for Biofuels. ,vol. 10, pp. 1- 10 ,(2017) , 10.1186/S13068-017-0846-5
Emmanuel Damilano Dutra, Fernando Almeida Santos, Bárbara Ribeiro Alves Alencar, Alexandre Libanio Silva Reis, Raquel de Fatima Rodrigues de Souza, Katia Aparecida da Silva Aquino, Marcos Antônio Morais Jr, Rômulo Simões Cezar Menezes, Alkaline hydrogen peroxide pretreatment of lignocellulosic biomass: status and perspectives Biomass Conversion and Biorefinery. ,vol. 8, pp. 225- 234 ,(2018) , 10.1007/S13399-017-0277-3
Jorge Rencoret, Antonio Pereira, José C. del Río, Ángel T. Martínez, Ana Gutiérrez, Delignification and Saccharification Enhancement of Sugarcane Byproducts by a Laccase-Based Pretreatment ACS Sustainable Chemistry & Engineering. ,vol. 5, pp. 7145- 7154 ,(2017) , 10.1021/ACSSUSCHEMENG.7B01332
Hyeong Rae Lee, Hun Wook Lee, Youn-Woo Lee, Romas J. Kazlauskas, Tai Hyun Park, Improved pretreatment of yellow poplar biomass using hot compressed water and enzymatically-generated peracetic acid Biomass & Bioenergy. ,vol. 105, pp. 190- 196 ,(2017) , 10.1016/J.BIOMBIOE.2017.07.004
Tamas Fodi, Christos Didaskalou, Jozsef Kupai, Gyorgy T. Balogh, Peter Huszthy, Gyorgy Szekely, Nanofiltration-Enabled In Situ Solvent and Reagent Recycle for Sustainable Continuous-Flow Synthesis. Chemsuschem. ,vol. 10, pp. 3435- 3444 ,(2017) , 10.1002/CSSC.201701120