A Dispersion Modeling Study of Major VOCs from Non‐Point Emission Sources in the Urban Atmosphere

作者: M.-S. Kim , J. H. Kim , H.-S. Park , Y. S. Sun , J. Yi

DOI: 10.1002/ELSC.200620175

关键词:

摘要: To assist with the understanding and solving of toxic air pollutant problems in urban areas, an atmospheric dispersion model, SKYDM, was developed three preprocessors (meteorology, emission, topography), a physical process chemical decay term based on NO x -O 3 -RH photochemistry actual atmosphere. SKYDM can work multicomponents single model run, as well compound run produces 2D meteorological field results due to integration approach. The present study aims develop evaluate at local spatial scales, short term. A comparative is conducted estimate effects parameters defining applicability limits models examine approach methodology. All simulations are for volatile organic compounds (VOCs) such BTXS (Benzene, Toluene, Xylene, Styrene) emitted from non-point sources, located 151 villages seven divisions, northeastern portion Seoul, Korea, eight different data sets during 2002. Modeled toluene concentrations compared those observed ten monitoring sites. main findings follows: (a) Model uncertainties obviously caused by limitations conditions emission topographical information, removal processes, user errors or application skills - comparatively significant parameter pollutants, (b) indicated correlation between observations (c) showed potential useful tool assessing quality areas. In further work, will be upgraded improving algorithm fully detailed input evaluated comparison other Gaussian models.

参考文章(21)
Dag Kappes, Kirsten Rasmussen, Prioritisation of existing biocidal active substances in the European Union Environmental Science & Policy. ,vol. 6, pp. 521- 532 ,(2003) , 10.1016/J.ENVSCI.2003.07.002
Kwangsam Na, Yong Pyo Kim, Kil Choo Moon, Diurnal characteristics of volatile organic compounds in the Seoul atmosphere Atmospheric Environment. ,vol. 37, pp. 733- 742 ,(2003) , 10.1016/S1352-2310(02)00956-1
K Hughes, M.E Meek, M Walker, Health risk assessment of 1,3-butadiene as a Priority Substance in Canada. Chemico-Biological Interactions. ,vol. 135, pp. 109- 135 ,(2001) , 10.1016/S0009-2797(01)00173-9
Ben-Jei Tsuang, Chien-Lung Chen, Chung-Hsien Lin, Man-Ting Cheng, Ying-I Tsai, Chia-Pin Chio, Rong-Chang Pan, Pei-Hsuan Kuo, Quantification on the source/receptor relationship of primary pollutants and secondary aerosols by a Gaussian plume trajectory model: Part II. Case study Atmospheric Environment. ,vol. 37, pp. 3981- 3991 ,(2003) , 10.1016/S1352-2310(03)00472-2
R.G Derwent, M.E Jenkin, S.M Saunders, M.J Pilling, P.G Simmonds, N.R Passant, G.J Dollard, P Dumitrean, A Kent, Photochemical ozone formation in north west Europe and its control Atmospheric Environment. ,vol. 37, pp. 1983- 1991 ,(2003) , 10.1016/S1352-2310(03)00031-1
M Placet, Emissions of ozone precursors from stationary sources: a critical review Atmospheric Environment. ,vol. 34, pp. 2183- 2204 ,(2000) , 10.1016/S1352-2310(99)00464-1
Michael Möllmann-Coers, Dieter Klemp, Katja Mannschreck, Franz Slemr, Statistical study of the diurnal variation of modeled and measured NMHC contributions Atmospheric Environment. ,vol. 36, pp. 109- 122 ,(2002) , 10.1016/S1352-2310(02)00217-0