Estimates of power plant NOx emissions and lifetimes from OMI NO2 satellite retrievals

作者: Benjamin de Foy , Zifeng Lu , David G. Streets , Lok N. Lamsal , Bryan N. Duncan

DOI: 10.1016/J.ATMOSENV.2015.05.056

关键词:

摘要: Isolated power plants with well characterized emissions serve as an ideal test case of methods to estimate using satellite data. In this study we evaluate the Exponentially-Modified Gaussian (EMG) method and box model based on mass balance for estimating known NOx from retrievals made by Ozone Monitoring Instrument (OMI). We consider 29 in USA which have large plumes that do not overlap other sources data Continuous Emission System (CEMS). This enables us identify constraints required methods, such wind use how calculate background values. found lifetimes estimated are too short be representative chemical lifetime. Instead, introduce a separate lifetime parameter account discrepancy between estimates real those theory would predict. terms emissions, EMG averages multiple years give accurate results, whereas gave results individual ozone seasons.

参考文章(43)
V. E. Fioletov, C. A. McLinden, N. Krotkov, M. D. Moran, K. Yang, Estimation of SO2 emissions using OMI retrievals Geophysical Research Letters. ,vol. 38, ,(2011) , 10.1029/2011GL049402
B. Mijling, R. J. van der A, Using daily satellite observations to estimate emissions of short-lived air pollutants on a mesoscopic scale Journal of Geophysical Research: Atmospheres. ,vol. 117, pp. n/a- n/a ,(2012) , 10.1029/2012JD017817
Raymond M Hoff, Sundar A Christopher, None, Remote sensing of particulate pollution from space: have we reached the promised land? Journal of The Air & Waste Management Association. ,vol. 59, pp. 645- 675 ,(2009) , 10.3155/1047-3289.59.6.645
L. C. Valin, A. R. Russell, R. C. Cohen, Variations of OH radical in an urban plume inferred from NO2 column measurements Geophysical Research Letters. ,vol. 40, pp. 1856- 1860 ,(2013) , 10.1002/GRL.50267
S‐W Kim, A Heckel, SA McKeen, GJ Frost, E‐Y Hsie, MK Trainer, A Richter, JP Burrows, SE Peckham, GA Grell, None, Satellite-observed U.S. power plant NOxemission reductions and their impact on air quality Geophysical Research Letters. ,vol. 33, ,(2006) , 10.1029/2006GL027749
S.-W. Kim, A. Heckel, G. J. Frost, A. Richter, J. Gleason, J. P. Burrows, S. McKeen, E.-Y. Hsie, C. Granier, M. Trainer, NO2 columns in the western United States observed from space and simulated by a regional chemistry model and their implications for NOx emissions Journal of Geophysical Research. ,vol. 114, ,(2009) , 10.1029/2008JD011343
S. Beirle, K. F. Boersma, U. Platt, M. G. Lawrence, T. Wagner, Megacity Emissions and Lifetimes of Nitrogen Oxides Probed from Space Science. ,vol. 333, pp. 1737- 1739 ,(2011) , 10.1126/SCIENCE.1207824
J.P. Veefkind, I. Aben, K. McMullan, H. Förster, J. de Vries, G. Otter, J. Claas, H.J. Eskes, J.F. de Haan, Q. Kleipool, M. van Weele, O. Hasekamp, R. Hoogeveen, J. Landgraf, R. Snel, P. Tol, P. Ingmann, R. Voors, B. Kruizinga, R. Vink, H. Visser, P.F. Levelt, TROPOMI on the ESA Sentinel-5 Precursor: A GMES mission for global observations of the atmospheric composition for climate, air quality and ozone layer applications Remote Sensing of Environment. ,vol. 120, pp. 70- 83 ,(2012) , 10.1016/J.RSE.2011.09.027
A. R. Russell, L. C. Valin, R. C. Cohen, Trends in OMI NO 2 observations over the United States: effects of emission control technology and the economic recession Atmospheric Chemistry and Physics. ,vol. 12, pp. 12197- 12209 ,(2012) , 10.5194/ACP-12-12197-2012
T. Stavrakou, J.-F. Müller, K. F. Boersma, R. J. van der A, J. Kurokawa, T. Ohara, Q. Zhang, Key chemical NOx sink uncertainties and how they influence top-down emissions of nitrogen oxides Atmospheric Chemistry and Physics. ,vol. 13, pp. 9057- 9082 ,(2013) , 10.5194/ACP-13-9057-2013