Exploiting satellite earth observation to quantify current global oceanic DMS flux and its future climate sensitivity

作者: P. E. Land , J. D. Shutler , T. G. Bell , M. Yang

DOI: 10.1002/2014JC010104

关键词:

摘要: We used coincident Envisat RA2 and AATSR temperature wind speed data from 2008/2009 to calculate the global net sea-air flux of dimethyl sulfide (DMS), which we estimate be 19.6 Tg S a−1. Our monthly calculations are compared open ocean eddy correlation measurements DMS 10 recent cruises, with a root mean square difference 3.1 μmol m−2 day−1. In sensitivity analysis, varied temperature, salinity, surface speed, aqueous concentration, using fixed changes as well CMIP5 model output. The range in future climate scenarios is discussed. predicts reduction that this will decrease annual by 22% over 25 years. Concurrent concentration increase much smaller amounts. effect all modelled year predictions was 19% flux. had significant regional effects, some positive (Southern Ocean, North Atlantic, Northwest Pacific) negative (isolated regions along Equator Indian Ocean). Using satellite-detected coverage coccolithophore blooms, our their contribution Atlantic emissions suggests coccolithophores contribute only small percentage estimate, but may more important summertime northeast Atlantic.

参考文章(58)
Rafel Simó, Jordi Dachs, Global ocean emission of dimethylsulfide predicted from biogeophysical data Global Biogeochemical Cycles. ,vol. 16, pp. 26-1- 26-10 ,(2002) , 10.1029/2001GB001829
Philip Cameron-Smith, Scott Elliott, Mathew Maltrud, David Erickson, Oliver Wingenter, Changes in dimethyl sulfide oceanic distribution due to climate change Geophysical Research Letters. ,vol. 38, ,(2011) , 10.1029/2011GL047069
B. J. Huebert, B. W. Blomquist, M. X. Yang, S. D. Archer, P. D. Nightingale, M. J. Yelland, J. Stephens, R. W. Pascal, B. I. Moat, Linearity of DMS transfer coefficient with both friction velocity and wind speed in the moderate wind speed range Geophysical Research Letters. ,vol. 37, ,(2010) , 10.1029/2009GL041203
Martí Galí, Rafel Simó, Maria Vila-Costa, Clara Ruiz-González, Josep M. Gasol, Patricia Matrai, Diel patterns of oceanic dimethylsulfide (DMS) cycling: Microbial and physical drivers Global Biogeochemical Cycles. ,vol. 27, pp. 620- 636 ,(2013) , 10.1002/GBC.20047
Brent G. T. Else, Tim N. Papakyriakou, Mats A. Granskog, John J. Yackel, Observations of sea surface fCO2 distributions and estimated air‐sea CO2 fluxes in the Hudson Bay region (Canada) during the open water season Journal of Geophysical Research. ,vol. 113, ,(2008) , 10.1029/2007JC004389
Katharina D. Six, Silvia Kloster, Tatiana Ilyina, Stephen D. Archer, Kai Zhang, Ernst Maier-Reimer, Global warming amplified by reduced sulphur fluxes as a result of ocean acidification Nature Climate Change. ,vol. 3, pp. 975- 978 ,(2013) , 10.1038/NCLIMATE1981
Craig J. Donlon, Matthew Martin, John Stark, Jonah Roberts-Jones, Emma Fiedler, Werenfrid Wimmer, The Operational Sea Surface Temperature and Sea Ice Analysis (OSTIA) system Remote Sensing of Environment. ,vol. 116, pp. 140- 158 ,(2012) , 10.1016/J.RSE.2010.10.017
Robert J. Charlson, James E. Lovelock, Meinrat O. Andreae, Stephen G. Warren, Oceanic phytoplankton, atmospheric sulphur, cloud albedo and climate Nature. ,vol. 326, pp. 655- 661 ,(1987) , 10.1038/326655A0
J. R. Gunson, S. A. Spall, T. R. Anderson, A. Jones, I. J. Totterdell, M. J. Woodage, Climate sensitivity to ocean dimethylsulphide emissions Geophysical Research Letters. ,vol. 33, ,(2006) , 10.1029/2005GL024982
A. D. Clarke, S. Freitag, R. M. C. Simpson, J. G. Hudson, S. G. Howell, V. L. Brekhovskikh, T. Campos, V. N. Kapustin, J. Zhou, Free troposphere as a major source of CCN for the equatorial pacific boundary layer: long-range transport and teleconnections Atmospheric Chemistry and Physics. ,vol. 13, pp. 7511- 7529 ,(2013) , 10.5194/ACP-13-7511-2013