Dynamics of inter- and intrastrand hole transport in DNA hairpins.
作者： Frederick D. Lewis , Xiaobing Zuo , Jianqin Liu , Ryan T. Hayes , Michael R. Wasielewski
DOI: 10.1021/JA0177859
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摘要: The dynamics of photoinduced electron transfer has been investigated in DNA hairpins possessing a stilbenedicarboxamide (Sa) acceptor, guanine (G) primary donor, and two adjacent guanines (GG) as secondary donors. Hole transport from G to GG across single A is more rapid than AA or T by factors 20 ± 7 40 15, respectively. Intrastrand hole interstrand factor 3.
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