Electronic Structure of Atomically Precise Graphene Nanoribbons
作者： Pascal Ruffieux , Jinming Cai , Nicholas C. Plumb , Luc Patthey , Deborah Prezzi
DOI: 10.1021/NN3021376
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摘要: Some of the most intriguing properties graphene are predicted for specifically designed nanostructures such as nanoribbons. Functionalities far beyond those known from extended systems include electronic band gap variations related to quantum confinement and edge effects, well localized spin-polarized states specific geometries. The inability produce with needed precision, however, has so hampered verification properties. Here, we report on dispersion occupied bands atomically precise nanoribbons fabricated via on-surface synthesis. Angle-resolved photoelectron spectroscopy scanning tunneling data armchair width N = 7 supported Au(111) reveal a 2.3 eV, an effective mass 0.21 m0 at top valence band, energy-dependent charge carrier velocity reaching 8.2 × 105 m/s in li...
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Xueliang Li, Yongtang Shi, Ivan Gutman, The Chemical Connection Springer, New York, NY. pp. 11- 17 ,(2012) , 10.1007/978-1-4614-4220-2_2
A. K. Geim, D. Jiang, S. V. Morozov, Y. Zhang, K. S. Novoselov, S. V. Dubonos, Room-temperature electric field effect and carrier-type inversion in graphene films arXiv: Mesoscale and Nanoscale Physics. ,(2004)
Thomas Seyller, Taisuke Ohta, Eli Rotenberg, K. Horn, Aaron Bostwick, Experimental Determination of the Spectral Function of Graphene arXiv: Strongly Correlated Electrons. ,(2006)
Kazuyoshi Tanaka, Tokio Yamabe, Electronic Structure of Conductive Conjugated Systems and Their Physicochemical Properties Advances in Quantum Chemistry. ,vol. 17, pp. 251- 284 ,(1985) , 10.1016/S0065-3276(08)60304-4
Richard M. Martin, Electronic Structure: Basic Theory and Practical Methods ,(2004)
Eric Clar, The aromatic sextet ,(1972)
Tobias Wassmann, Ari P. Seitsonen, A. Marco Saitta, Michele Lazzeri, Francesco Mauri, Clar's Theory, STM Images, and Geometry of Graphene Nanoribbons arXiv: Materials Science. ,(2010) , 10.1021/JA909234Y
Tamar Stein, Helen Eisenberg, Leeor Kronik, Roi Baer, Fundamental Gaps in Finite Systems from Eigenvalues of a Generalized Kohn-Sham Method Physical Review Letters. ,vol. 105, pp. 266802- ,(2010) , 10.1103/PHYSREVLETT.105.266802
Fabian H. L. Essler, Holger Frahm, Frank Göhmann, Andreas Klümper, Vladimir E. Korepin, The one-dimensional Hubbard model odhm. ,(2005) , 10.1017/CBO9780511534843
Horst rer. nat. habil. Sachs, Siemion Fajtlowicz, Peter E. Pd Dr. rer. nat. habil. John, On Maximum Matchings and Eigenvalues of Benzenoid Graphs Croatica Chemica Acta. ,vol. 78, pp. 195- 201 ,(2005)