Multidimensional high harmonic spectroscopy

作者: Barry D Bruner , Hadas Soifer , Dror Shafir , Valeria Serbinenko , Olga Smirnova

DOI: 10.1088/0953-4075/48/17/174006

关键词:

摘要: High harmonic generation (HHG) has opened up a new frontier in ultrafast science where attosecond time resolution and Angstrom spatial are accessible single measurement. However, reconstructing the dynamics under study is limited by multiple degrees of freedom involved strong field interactions. In this paper we describe class measurement schemes for resolving dynamics, integrating perturbative nonlinear optics with strong-field physics. These approaches serve as basis multidimensional high spectroscopy. Specifically, show that spectroscopy can measure tunnel ionization precision, resolves interference between channels. addition, how HHG function type lock-in amplifier Similar to multi-dimensional optical have resolved correlated femtosecond reveals underlying complex behind scale phenomena.

参考文章(61)
Jennifer P. Ogilvie, Kevin J. Kubarych, Chapter 5 Multidimensional Electronic and Vibrational Spectroscopy: An Ultrafast Probe of Molecular Relaxation and Reaction Dynamics Advances in Atomic Molecular and Optical Physics. ,vol. 57, pp. 249- 321 ,(2009) , 10.1016/S1049-250X(09)57005-X
Martin Zanni, Peter Hamm, Concepts and Methods of 2D Infrared Spectroscopy ,(2011)
Olga Smirnova, Misha Ivanov, Multielectron High Harmonic Generation: Simple Man on a Complex Plane arXiv: Atomic Physics. pp. 201- 256 ,(2014) , 10.1002/9783527677689.CH7
D Shafir, Y Mairesse, H J Wörner, K Rupnik, D M Villeneuve, P B Corkum, N Dudovich, Probing the symmetry of atomic wavefunctions from the point of view of strong field-driven electrons New Journal of Physics. ,vol. 12, pp. 073032- ,(2010) , 10.1088/1367-2630/12/7/073032
F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, S. Stagira, Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver Optics Letters. ,vol. 34, pp. 3125- 3127 ,(2009) , 10.1364/OL.34.003125
Cosmin I. Blaga, Junliang Xu, Anthony D. DiChiara, Emily Sistrunk, Kaikai Zhang, Pierre Agostini, Terry A. Miller, Louis F. DiMauro, C. D. Lin, Imaging ultrafast molecular dynamics with laser-induced electron diffraction Nature. ,vol. 483, pp. 194- 197 ,(2012) , 10.1038/NATURE10820
Eleftherios Goulielmakis, Zhi-Heng Loh, Adrian Wirth, Robin Santra, Nina Rohringer, Vladislav S. Yakovlev, Sergey Zherebtsov, Thomas Pfeifer, Abdallah M. Azzeer, Matthias F. Kling, Stephen R. Leone, Ferenc Krausz, Real-time observation of valence electron motion Nature. ,vol. 466, pp. 739- 743 ,(2010) , 10.1038/NATURE09212
M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, F. Krausz, Attosecond real-time observation of electron tunnelling in atoms Nature. ,vol. 446, pp. 627- 632 ,(2007) , 10.1038/NATURE05648
O. Raz, O. Pedatzur, B. D. Bruner, N. Dudovich, Spectral caustics in attosecond science Nature Photonics. ,vol. 6, pp. 170- 173 ,(2012) , 10.1038/NPHOTON.2011.353
Sarah M. Gallagher Faeder, David M. Jonas, Two-Dimensional Electronic Correlation and Relaxation Spectra: Theory and Model Calculations Journal of Physical Chemistry A. ,vol. 103, pp. 10489- 10505 ,(1999) , 10.1021/JP9925738