Characterization of Size-Fractionated Aerosol from the Jungfraujoch (3580 m asl) Using Total Reflection X-Ray Fluorescence (TXRF)
作者： Niklaus Streit , Ernest Weingartner , Christoph Zellweger , Margit Schwikowski , Heinz W. Gäggeler
DOI: 10.1080/03067310008034114
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摘要: Abstract During three field campaigns at the Jungfraujoch High Alpine Research Station, Switzerland, size-fractionated aerosol was collected using a cascade impactor. The particles were impacted on silicon oil-coated quartz sampling substrates. actual analysis then performed directly these substrates total reflection X-ray fluorescence. resulting size distributions of 16 elements (S, Cl, K, Ca, Ti, Mn, Fe, Cu, Zn, Se, Br, Rb, Sr, Y, Zr, Pb) investigated to determine best cut-off diameter distinguish between geogenic and anthropogenic particles. obtained 1 μm is an important parameter in current world-wide measurements under auspices World Meteorological Organization's Global Atmosphere Watch project.
sci-hub.se 参考文章(36)
Reinhold Klockenkamper, Total-Reflection X-Ray Fluorescence Analysis ,(1996)
Kurt F.J. Heinrich, Advances in X-Ray Analysis ,(1978)
Y. Yoneda, T. Horiuchi, Optical flats for use in x-ray spectrochemical microanalysis. Review of Scientific Instruments. ,vol. 42, pp. 1069- 1070 ,(1971) , 10.1063/1.1685282
W. P. Kelly, P. H. McMurry, Measurement of Particle Density by Inertial Classification of Differential Mobility Analyzer–Generated Monodisperse Aerosols Aerosol Science and Technology. ,vol. 17, pp. 199- 212 ,(1992) , 10.1080/02786829208959571
D. J. Leland, D. B. Bilbrey, D. E. Leyden, Peter. Wobrauschek, Hannes. Aiginger, Hans. Puxbaum, Analysis of aerosols using total reflection x-ray spectrometry Analytical Chemistry. ,vol. 59, pp. 1911- 1914 ,(1987) , 10.1021/AC00142A005
J. E. Penner, R. J. Charlson, S. E. Schwartz, J. M. Hales, N. S. Laulainen, L. Travis, R. Leifer, T. Novakov, J. Ogren, L. F. Radke, Quantifying and Minimizing Uncertainty of Climate Forcing by Anthropogenic Aerosols Bulletin of the American Meteorological Society. ,vol. 75, pp. 375- 400 ,(1994) , 10.1175/1520-0477(1994)075<0375:QAMUOC>2.0.CO;2
R. Dams, J. De Jonge, Chemical composition of Swiss aerosols from the Jungfraujoch Atmospheric Environment. ,vol. 10, pp. 1079- 1084 ,(1976) , 10.1016/0004-6981(76)90117-7
Ina Tegen, Peter Hollrig, Mian Chin, Inez Fung, Daniel Jacob, Joyce Penner, Contribution of different aerosol species to the global aerosol extinction optical thickness: Estimates from model results Journal of Geophysical Research. ,vol. 102, pp. 23895- 23915 ,(1997) , 10.1029/97JD01864
S.V. Hering, S.K. Friedlander, Origins of aerosol sulfur size distributions in the Los Angeles basin Atmospheric Environment. ,vol. 16, pp. 2647- 2656 ,(1982) , 10.1016/0004-6981(82)90346-8
S. E. Schwartz, M. O. Andreae, Uncertainty in Climate Change Caused by Aerosols Science. ,vol. 272, pp. 1121- 1121 ,(1996) , 10.1126/SCIENCE.272.5265.1121