Study of C60/Au(110)-p(6 × 5) Reconstruction from In-Plane X-Ray Diffraction Data

作者: M. Pedio , R. Felici , X. Torrelles , P. Rudolf , M. Capozi

DOI: 10.1103/PHYSREVLETT.85.1040

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摘要: Fullerene molecules absorbed on the highly anisotropic Au(110)-p(1x2) surface induce an ordered p(6x5) superstructure that has been solved by applying 2D "direct methods" difference sum function to x-ray diffraction data set. We found C (60)-gold interface is structurally much more complex than one previously suggested scanning tunneling microscopy [J. K. Gimzewski, S. Modesti, and R. Schlittler, Phys. Rev. Lett. 72, 1036 (1994)]. Indeed a large fraction of Au atoms are displaced from their original positions producing microscopic pits may accommodate fullerene molecules.

参考文章(21)
R. J. Wilson, G. Meijer, D. S. Bethune, R. D. Johnson, D. D. Chambliss, M. S. de Vries, H. E. Hunziker, H. R. Wendt, Imaging C 60 clusters on a surface using a scanning tunnelling microscope Nature. ,vol. 348, pp. 621- 622 ,(1990) , 10.1038/348621A0
G. Gensterblum, K. Hevesi, B.-Y. Han, L.-M. Yu, J.-J. Pireaux, P. A. Thiry, R. Caudano, A.-A. Lucas, D. Bernaerts, S. Amelinckx, G. Van Tendeloo, G. Bendele, T. Buslaps, R. L. Johnson, M. Foss, R. Feidenhans’l, G. Le Lay, Growth mode and electronic structure of the epitaxial C60(111)/GeS(001) interface. Physical Review B. ,vol. 50, pp. 11981- 11995 ,(1994) , 10.1103/PHYSREVB.50.11981
A.V. Hamza, M. Balooch, The chemisorption of C60 on Si(100)-(2×1) Chemical Physics Letters. ,vol. 201, pp. 404- 408 ,(1993) , 10.1016/0009-2614(93)85092-3
P.A. Brühwiler, A.J. Maxwell, P. Baltzer, S. Andersson, D. Arvanitis, L. Karlsson, N. Mårtensson, Vibronic coupling in the photoemission bands of condensed C60 Chemical Physics Letters. ,vol. 279, pp. 85- 91 ,(1997) , 10.1016/S0009-2614(97)00949-4
Petra Rudolf, Mark S Golden, Paul A Brühwiler, Studies of fullerenes by the excitation, emission, and scattering of electrons Journal of Electron Spectroscopy and Related Phenomena. ,vol. 100, pp. 409- 433 ,(1999) , 10.1016/S0368-2048(99)00058-4
A. J. Maxwell, P. A. Brühwiler, D. Arvanitis, J. Hasselström, M. K.-J. Johansson, N. Mårtensson, Electronic and geometric structure of C 60 on Al(111) and Al(110) Physical Review B. ,vol. 57, pp. 7312- 7326 ,(1998) , 10.1103/PHYSREVB.57.7312
R. Fasel, P. Aebi, R. G. Agostino, D. Naumović, J. Osterwalder, A. Santaniello, L. Schlapbach, Orientation of adsorbed C60 molecules determined via x-ray photoelectron diffraction. Physical Review Letters. ,vol. 76, pp. 4733- 4736 ,(1996) , 10.1103/PHYSREVLETT.76.4733
P. W. Murray, M. Ø. Pedersen, E. Lægsgaard, I. Stensgaard, F. Besenbacher, Growth of C 60 on Cu(110) and Ni(110) surfaces: C 60 -induced interfacial roughening Physical Review B. ,vol. 55, pp. 9360- 9363 ,(1997) , 10.1103/PHYSREVB.55.9360
J. K. Gimzewski, S. Modesti, R. R. Schlittler, Cooperative self-assembly of Au atoms and C60 on Au(110) surfaces. Physical Review Letters. ,vol. 72, pp. 1036- 1039 ,(1994) , 10.1103/PHYSREVLETT.72.1036
A. J. Maxwell, P. A. Brühwiler, A. Nilsson, N. Mårtensson, P. Rudolf, Photoemission, autoionization, and x-ray-absorption spectroscopy of ultrathin-film C60 on Au(110). Physical Review B. ,vol. 49, pp. 10717- 10725 ,(1994) , 10.1103/PHYSREVB.49.10717